I wonder if the 'bar' used was not accurately round, or perhaps hexagonal? I have found examples of hex bar in which the AF dimensions were out. (AF = across flats)
I agree with the 'don't bin it' advice. There are many jobs where the concentricity of the chuck is not critical, and many off-the-shelf components where the parts are not concentric from new. Things like hydraulic pipe fittings, where the flats are not always in line with the threads or the bore.
But before you consider your next move, it would be useful to do a series of checks using (eg) silver steel bars of different sizes, noting the run-out of each. This would give you info to work out whether the scroll was bad in parts, or a jaw was distorted. It would be no use grinding the jaws to get it back on form, if the scroll was bruised on one (or more) places. The next time you used it with a different size, it would show a new eccentricity.
Regards, Tim